[1]韩梦丽,王建海,沈岳松.光热催化二氧化碳还原研究综述[J].中国材料进展,2024,43(07):050-59.
 HAN Mengli,WANG Jianhai,SHEN Yuesong.A Review of Photothermal Catalyzed CO2 Reduction Research[J].MATERIALS CHINA,2024,43(07):050-59.
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光热催化二氧化碳还原研究综述()
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中国材料进展[ISSN:1674-3962/CN:61-1473/TG]

卷:
43
期数:
2024年第07期
页码:
050-59
栏目:
出版日期:
2024-07-30

文章信息/Info

Title:
A Review of Photothermal Catalyzed CO2 Reduction Research
文章编号:
1674—3962 (2019)04-0000-00
作者:
韩梦丽王建海沈岳松
南京工业大学材料科学与工程学院,江苏 南京 211816
Author(s):
HAN MengliWANG JianhaiSHEN Yuesong
College of Materials Science and Engineering, Nanjing Tech University, Nanjing 211816, China
关键词:
光热催化二氧化碳还原催化机理优化设计工业化应用
Keywords:
光热催化二氧化碳还原催化机理优化设计工业化应用
分类号:
O643.31
文献标志码:
A
摘要:
能源短缺与环境污染是当今世界发展的两大难题。以化石能源为主体的能源消耗不仅造成严重的能源危机,同时产生大量的CO2,造成温室效应,引发广泛的环境危机。因此,降碳减污成为全球发展的重大战略需求。其中,CO2资源化利用不仅可以减少环境污染,其还原产生的碳基产物往往是重要的化工中间体,具有巨大的应用价值,因此,CO2还原制备碳基产物成为当前能源与环境领域研究的热点。目前,CO2催化还原的方法主要有热催化、光催化、电催化、光热催化和光电催化等,其中光热耦合的光驱动光热协同催化技术,不仅克服了单一催化技术存在的不足,同时充分发挥二者的优势,在低(无)能耗的条件下实现高效、选择性的还原CO2制备碳基化合物,是一种理想的还原途径。针对光热催化的分类、机理及光热催化二氧化碳还原催化剂的优化设计,分别做出了概括、总结;并阐述了光热催化二氧化碳还原的工业化应用及存在问题;最后对光热催化二氧化碳的未来发展进行展望。
Abstract:
Energy shortage and environmental pollution are two major problems in the development of the world. Energy consumption mainly based on fossil energy not only causes a serious energy crisis, but also produces a large amount of CO2, which causes the greenhouse effect and triggers a wide range of environmental crises. Therefore, carbon reduction and pollution reduction have become a major strategic need for global development. Among them, the utilization of CO2 resources can not only reduce environmental pollution, but also the carbon-based products generated by its reduction are often important chemical intermediates with great application value, therefore, the preparation of carbon-based products by CO2 reduction has become a hotspot of current research in the field of energy and environment. At present, CO2 catalytic reduction methods mainly include thermal catalysis, photocatalysis, electrocatalysis, photothermal catalysis and photoelectrocatalysis, etc. Among them, the photothermal coupling of light-driven photothermal synergistic catalytic technology not only overcomes the deficiencies of a single catalytic technology, but also gives full play to the advantages of the two, and realizes the preparation of carbon-based compounds from CO2 reduction with high efficiency and selectivity under the condition of low (no) energy consumption, which is an ideal reduction pathway It is an ideal reduction pathway. The classification, mechanism and application of photothermal catalysis for CO2 reduction are outlined, summarized and expressed respectively; the optimal design of photothermal catalytic CO2 catalysts is discussed; and finally, the future development of photothermal catalytic CO2 is envisioned.
更新日期/Last Update: 2024-06-26